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Herein, a new class of robust bicontinuous elastomer–metal foam composites with highly tunable mechanical stiffness is proposed, fabricated, characterized, and demonstrated. The smart composite is a bicontinuous network of two foams, one metallic made of a low melting point alloy (LMPA) and the other elastomeric made of polydimethylsiloxane (PDMS). The stiffness of the composite can be tuned by inducing phase changes in its LMPA component. Below the melting point of the LMPA, Young's modulus of the smart composites is ≈1 GPa, whereas above the melting point of the LMPA it is ≈1 MPa. Thus, a sharp stiffness change of ≈1000× can be realized through the proposed bicontinuous foam composite structure, which is higher than all available robust smart composites. Effective medium theory is also used to predict the Young's modulus of the bicontinuous smart composites, which generates reasonable agreement with experimentally measured Young's modulus of the smart composites. Finally, the use of these smart materials as a smart joint in a robotic arm is also demonstrated.
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Abstract Recently, a novel concept to realize dynamically tunable dry adhesion via subsurface stiffness modulation (SSM) in a composite core–shell structure has been introduced and demonstrated for gripping and release of objects. Here, a variant form of the composite core–shell design is proposed to significantly improve the performance of dynamically tunable dry adhesion in terms of activation time and activation voltage. Specifically, composite pillars with an embedded microfluidic channel filled with a low melting point alloy (LMPA) are fabricated, and the adhesion of the pillars is characterized as a function of LMPA state: either melted or solid. The effects of the thickness and in‐plane pattern of the LMPA channel, as well as the depth at which it is embedded on tunable adhesion are investigated. Experiments show that the effective adhesion strength can be reduced up to 50%, equivalent to a 2× change in dry adhesion when the LMPA is melted. Finite element analysis of the stress distribution change under SSM shows that the experimentally observed tunable adhesion is primarily due to stiffness change close to the interface. In addition, two technology demonstrations of composite pillars picking and releasing objects with fast activation (≈1 s) and low activation voltages (≈1 V) are included.
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Robust Three‐Component Elastomer–Particle–Fiber Composites with Tunable Properties for Soft Robotics
Materials with tunable properties, especially dynamically tunable stiffness, have been of great interest for the field of soft robotics. Herein, a novel design concept of robust three‐component elastomer–particle–fiber composite system with tunable mechanical stiffness and electrical conductivity is introduced. These smart materials are capable of changing their mechanical stiffness rapidly and reversibly when powered with electrical current. One implementation of the composite system demonstrated here is composed of a polydimethylsiloxane (PDMS) matrix, Field's metal (FM) particles, and nickel‐coated carbon fibers (NCCF). It is demonstrated that the mechanical stiffness and the electrical conductivity of the composite are highly tunable and dependent on the volume fraction of the three components and the temperature, and can be reasonably estimated using effective medium theory. Due to its superior electrical conductivity, Joule heating can be used as the activation mechanism to realize ≈20× mechanical stiffness changes in seconds. The performance of the composites is thermally and mechanically robust. The shape memory effect of these composites is also demonstrated. The combination of tunable mechanical and electrical properties makes these composites promising candidates for sensing and actuation applications for soft robotics.